Uing a converter software can get this done. Wondershare Video Converter for Mac is one of the many good converter.
You can convert .flv, .mov, .wmv, .mod .moi .mpg, .mpeg, JVC .tod, .m2t, AVI, ASF, VOB and other popular video formats to iMovie.
What's more, you will be attracted by the feature of creating video clips and merging videos. If you want to do more things about your movie, you can extract audios from video and save them as MP3s, so that you can listen them in you iPod.
IPOD
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